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NMR evidence of strongly correlated superconductivity in LiFeAs: Tuning toward a spin-density-wave ordering

L. Ma, J. Zhang, G. F. Chen, Weiqiang Yu

DOI 10.1103/PhysRevB.82.180501 · Physical Review B

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Abstract

In this Rapid Communication, we reported the results of NMR study on LiFeAs single crystals. We find a strong evidence of the low-temperature spin fluctuations; by changing sample preparation conditions, the system can be tuned toward a spin-density-wave (SDW) quantum-critical point. The detection of an interstitial Li(2) ion, possibly locating in the tetrahedral hole, suggests that the off-stoichiometry and/or lattice defect can probably account for the absence of the SDW ordering in LiFeAs. These facts show that LiFeAs is a strongly correlated system and the superconductivity is likely originated from the SDW fluctuations.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
LiFeAs

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17Pressure not reportedonset
LiFeAs

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

17Pressure not reportedonset
LiFeAs

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

10Pressure not reportedunknown
LiFeAs

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

18Pressure not reportedunknown

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