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Magnetic torque evidence for the Fulde-Ferrell-Larkin-Ovchinnikov state in the layered organic superconductor κ−(BEDT−TTF)2Cu(NCS)2

B. Bergk, A. Demuer, I. Sheikin, Y. Wang, J. Wosnitza, Y. Nakazawa, R. Lortz

DOI 10.1103/PhysRevB.83.064506 · Physical Review B

T1

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Abstract

We present magnetic-torque measurements of the organic superconductor κ-(BEDT-TTF)2Cu(NCS)2 for in-plane magnetic fields up to 32 T. In this layered two-dimensional compound the superconductivity can persist even in fields above the Pauli limit of about 21 T. There, a pronounced upturn of the upper-critical-field line occurs and the superconducting phase-transition line splits and forms an additional high-magnetic-field phase. κ-(BEDT-TTF)2Cu(NCS)2 is a spin-singlet superconductor; therefore, such a superconducting high-field phase beyond the Pauli limit can originate only from Cooper pairing with finite center-of-mass momentum. The mea-surements are discussed in connection with a Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state, in accordance with earlier specific-heat observations. The torque experiments allow us to investigate the high-magnetic-field phase diagram and the FFLO state of κ-(BEDT-TTF)2Cu(NCS)2 in great detail.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
κ-(BEDT-TTF)2Cu(NCS)2

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—Pressure not reportedunknown
CeCoIn5

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—Pressure not reportedunknown
λ-(BETS)2GaCl4

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—Pressure not reportedunknown
λ-(BETS)2FeCl4

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—Pressure not reportedunknown
(TMTSF)2PF6

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—Pressure not reportedunknown
(TMTSF)2ClO4

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—Pressure not reportedunknown
β"-(BEDT-TTF)2SF5CH2CF2SO3

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—Pressure not reportedunknown

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