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Calorimetric Evidence for a Fulde-Ferrell-Larkin-Ovchinnikov Superconducting State in the Layered Organic Superconductor κ−(BEDT−TTF)2Cu(NCS)2

R. Lortz, Y. Wang, A. Demuer, P. H. M. Böttger, B. Bergk, G. Zwicknagl, Y. Nakazawa, J. Wosnitza

DOI 10.1103/PhysRevLett.99.187002 · Physical Review Letters

T1

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Abstract

The specific heat of the layered organic superconductor κ−(BEDT−TTF)2Cu(NCS)2, where BEDT-TTF is bisethylenedithio-tetrathiafulvalene, has been studied in magnetic fields up to 28 T applied perpendicular and parallel to the superconducting layers. In parallel fields above 21 T, the superconducting transition becomes first order, which signals that the Pauli-limiting field is reached. Instead of saturating at this field value, the upper-critical-field increases sharply and a second first-order transition line appears within the superconducting phase. Our results give strong evidence that the phase, which separates the homogeneous superconducting state from the normal state is a realization of a Fulde-Ferrell-Larkin-Ovchinnikov state.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
κ-(BEDT-TTF)2Cu(NCS)2

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9.1Pressure not reportedonset

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