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High-resolution ac-calorimetry studies of the quasi-two-dimensional organic superconductor κ−(BEDT−TTF)2Cu(NCS)2

J. Müller, M. Lang, R. Helfrich, F. Steglich, T. Sasaki

DOI 10.1103/PhysRevB.65.140509 · Physical Review B

T1

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Abstract

We report high-resolution specific-heat measurements on the quasi-two-dimensional organic superconductor κ−(BEDT−TTF)2Cu(NCS)2, performed by using a sensitive ac-modulation technique. The main observations are (i) a discontinuity at Tc much in excess of what is expected for a weak-coupling BCS superconductor and (ii) a quasiparticle contribution to the specific heat with an exponentially weak temperature dependence at T≪Tc. The latter finding is incompatible with an order parameter that vanishes at certain parts of the Fermi surface. The data for T<~Tc can be well described by a strong-coupling extension of the BCS theory — the α-model — similar to what has been recently found for the κ−(BEDT−TTF)2Cu[N(CN)2]Br salt [Elsinger et al., Phys. Rev. Lett. 84, 6098 (2000)].

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
(BEDT-TTF)2Cu(NCS)2

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9Pressure not reportedonset
(BEDT-TTF)2Cu(N(CN)2)Br

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—Pressure not reportedunknown
(BEDT-TTF)2Cu(N(CN)2)Cl

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—Pressure not reportedunknown

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