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Superconductivity induced by U doping in the SmFeAsO system

Bo Huang, Jijun Yang, Jun Tang, Jiali Liao, Yuanyou Yang, Ning Liu, Gang Mu, Tao Hu, Xiaoping Shen, Donglai Feng

DOI 10.1103/PhysRevB.87.060501 · Physical Review B

T1

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Abstract

Through partial substitution of Sm by U in SmFeAsO, a different member of the family of iron-based superconductors was successfully synthesized. X-ray diffraction measurements show that the lattice constants along the a and c axes are both squeezed through U doping, indicating a successful substitution of U at the Sm site. The parent compound shows a strong resistivity anomaly near 150 K, associated with spin-density-wave instability. U doping suppresses this instability and leads to a transition to the superconducting state at temperatures up to 49 K. Magnetic measurements confirm the bulk superconductivity in this system. For the sample with a doping level of x=0.2, the external magnetic field suppresses the onset temperature very slowly, indicating a rather high upper critical field. In addition, the Hall effect measurements show that U clearly dopes electrons into the material.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
Sm1-xUxFeAsO

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49Pressure not reportedonset
Sm1-xUxFeAsO

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

46Pressure not reportedonset
Sm0.9U0.1FeAsO

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

47Pressure not reportedonset
Sm0.8U0.2FeAsO

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

49Pressure not reportedonset
Ln1-xThxFeAsO

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50Pressure not reportedunknown

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