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Evidence of unconventional low-frequency dynamics in the normal phase of Ba(Fe1−xRhx)2As2 iron-based superconductors

L. Bossoni, P. Carretta, W. P. Halperin, S. Oh, A. Reyes, P. Kuhns, P. C. Canfield

DOI 10.1103/PhysRevB.88.100503 · Physical Review B

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Abstract

This work presents 75As NMR spin-echo decay rate (1/T2) measurements in Ba(Fe1−xRhx)2As2 superconductors, for 0.041⩽x⩽0.094. It is shown that 1/T2 increases upon cooling, in the normal phase, suggesting the onset of an unconventional very low-frequency activated dynamic. The correlation times of the fluctuations and their energy barriers are derived. The motion is favored at large Rh content, while it is hindered by the application of a magnetic field perpendicular to the FeAs layers. The same dynamic is observed in the spin-lattice relaxation rate, in a quantitatively consistent manner. These results are discussed in the light of nematic fluctuations involving domain wall motion. The analogies with the behavior observed in the cuprates are also outlined.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
Ba(Fe1-xRhx)2As2

Archive — visibility unverified

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13.6Pressure not reportedunknown
Ba(Fe1-xRhx)2As2

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

22.4Pressure not reportedunknown
Ba(Fe1-xRhx)2As2

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

15.1Pressure not reportedunknown

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