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Effect of proton irradiation on the normal-state low-energy excitations of Ba(Fe1−xRhx)2As2 superconductors

M. Moroni, L. Gozzelino, G. Ghigo, M. A. Tanatar, R. Prozorov, P. C. Canfield, P. Carretta

DOI 10.1103/PhysRevB.96.094523 · Physical Review B

T1

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Abstract

We present a As75 nuclear magnetic resonance (NMR) and resistivity study of the effect of 5.5 MeV proton irradiation on the optimal electron doped (x=0.068) and overdoped (x=0.107) Ba(Fe1−xRhx)2As2 iron based superconductors. While the proton induced defects only mildly suppress the critical temperature and increase residual resistivity in both compositions, sizable broadening of the NMR spectra was observed in all the irradiated samples at low temperature. The effect is significantly stronger in the optimally doped sample where the Curie Weiss temperature dependence of the line width suggests the onset of ferromagnetic correlations coexisting with superconductivity at the nanoscale. 1/T2 measurements revealed that the energy barrier characterizing the low energy spin fluctuations of these compounds is enhanced upon proton irradiation, suggesting that the defects are likely slowing down the fluctuations between (0,π) and (π,0) nematic ground states.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
Ba(Fe1-xRhx)2As2

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23.3Pressure not reportedzero_resistance
Ba(Fe1-xRhx)2As2

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22.3Pressure not reportedzero_resistance
Ba(Fe1-xRhx)2As2

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13.7Pressure not reportedzero_resistance
Ba(Fe1-xRhx)2As2

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

12.9Pressure not reportedzero_resistance
Ba(Fe1-xRhx)2As2

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

23.3Pressure not reportedonset
Ba(Fe1-xRhx)2As2

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13.7Pressure not reportedonset
YBa2Cu3O7-δ

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown
Tl2Ba2CuO6+x

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown
Ba1-xKxFe2As2

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—Pressure not reportedunknown
Ba(Fe1-xCox)2As2

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—Pressure not reportedunknown
LaFeAsO1-xFx

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—Pressure not reportedunknown
Ba(Fe1-xRux)2As2

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—Pressure not reportedunknown

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