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Superconductivity proximate to antiferromagnetism in a copper-oxide monolayer grown on Bi2Sr2CaCu2O8+δ

Shuai Wang, Long Zhang, Fa Wang

DOI 10.1103/PhysRevB.97.035112 · Physical Review B

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Abstract

A nodeless superconducting (SC) gap was reported in a recent scanning tunneling spectroscopy experiment of a copper-oxide monolayer grown on a Bi2Sr2CaCu2O8+δ (Bi2212) substrate [Zhong et al., Sci. Bull. 61, 1239 (2016)], which is in stark contrast to the nodal d-wave pairing gap in the bulk cuprates. Motivated by this experiment, we first show with first-principles calculations that the tetragonal CuO (T-CuO) monolayer on the Bi2212 substrate is more stable than the commonly postulated CuO2 structure. The T-CuO monolayer is composed of two CuO2 layers sharing the same O atoms. The band structure is obtained by first-principles calculations, and its strong electron correlation is treated with the renormalized mean-field theory. We argue that one CuO2 sublattice is hole doped while the other sublattice remains half filled and may have antiferromagnetic (AF) order. The doped Cu sublattice can show d-wave SC; however, its proximity to the AF Cu sublattice induces a spin-dependent hopping, which splits the Fermi surface and may lead to a full SC gap. Therefore, the nodeless SC gap observed in the experiment could be accounted for by the d-wave SC proximity to an AF order, thus it is extrinsic rather than intrinsic to the CuO2 layers.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
CuO

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—Pressure not reportedunknown
Bi2Sr2CaCu2O8+δ

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown

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