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Superconductivity of single unit cell FeSe/SrTiO3(001): Substrate-surface superstructure dependence

Tomoaki Tanaka, Kenta Akiyama, Ryo Yoshino, Toru Hirahara

DOI 10.1103/PhysRevB.98.121410 · Physical Review B

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Abstract

We report the relationship between the surface superstructure of SrTiO3(001) (STO) substrates and the superconducting properties of single unit cell (1-UC) FeSe films using scanning tunneling microscopy/spectroscopy (STM/STS). Under reflection high-energy-electron diffraction observation, we controlled the periodicity of the STO surface to 2×1 and 2×2 and grew high-quality FeSe films. We found that the substrate periodicity can be imaged through the 1-UC FeSe from high-resolution STM observations and obtained clear evidence that the superconducting gap size depends on the surface periodicity (10–15 meV on 2×1, 12–17 meV on 2×2, and 9–13 meV for 2×1 domains on the 2×2 surface). Our results strongly suggest the important role of the film/substrate interface on high-temperature superconductivity.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
FeSe

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60Pressure not reportedonset
FeSe

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8Pressure not reportedunknown
FeSe

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—Pressure not reportedunknown

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