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Antiferroquadrupolar Ordering in a Pr-Based Superconductor PrIr2Zn20

T. Onimaru, K. T. Matsumoto, Y. F. Inoue, K. Umeo, T. Sakakibara, Y. Karaki, M. Kubota, T. Takabatake

DOI 10.1103/PhysRevLett.106.177001 · Physical Review Letters

T1

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Abstract

An antiferroquadrupolar ordering at TQ=0.11 K has been found in a Pr-based superconductor PrIr2Zn20. The measurements of specific heat and magnetization revealed the non-Kramers Γ3 doublet ground state with the quadrupolar degrees of freedom. The specific heat exhibits a sharp peak at TQ=0.11 K. The increment of TQ in magnetic fields and the anisotropic B−T phase diagram are consistent with the antiferroquadrupolar ordered state below TQ. The entropy release at TQ is only 20% of Rln2, suggesting that the quadrupolar fluctuations play a role in the formation of the superconducting pairs below Tc=0.05 K.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
PrIr2Zn20

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0.05Pressure unresolvedonset
LaIr2Zn20

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0.6Pressure not reportedunknown
PrOs4Sb12

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1.5Pressure not reportedunknown

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