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Electronic Correlations and Unconventional Spectral Weight Transfer in the High-Temperature Pnictide BaFe2−xCoxAs2 Superconductor Using Infrared Spectroscopy

A. A. Schafgans, S. J. Moon, B. C. Pursley, A. D. LaForge, M. M. Qazilbash, A. S. Sefat, D. Mandrus, K. Haule, G. Kotliar, D. N. Basov

DOI 10.1103/PhysRevLett.108.147002 · Physical Review Letters

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Abstract

We report an infrared optical study of the pnictide high-temperature superconductor BaFe1.84Co0.16As2 and its parent compound BaFe2As2. We demonstrate that electronic correlations are moderately strong and do not change across the spin-density wave transition or with doping. By examining the energy scale and direction of spectral weight transfer, we argue that Hund’s coupling J is the primary mechanism that gives rise to correlations.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
BaFe1.84Co0.16As2

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—Pressure not reportedunknown

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