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Feedback Effect on High-Energy Magnetic Fluctuations in the Model High-Temperature Superconductor HgBa2CuO4+δ Observed by Electronic Raman Scattering

Yuan Li, M. Le Tacon, M. Bakr, D. Terrade, D. Manske, R. Hackl, L. Ji, M. K. Chan, N. Barišić, X. Zhao, M. Greven, B. Keimer

DOI 10.1103/PhysRevLett.108.227003 · Physical Review Letters

T1

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Abstract

We use electronic Raman scattering to study the model single-layer cuprate superconductor HgBa2CuO4+δ. In an overdoped sample, we observe a pronounced amplitude enhancement of a high-energy peak related to two-magnon excitations in insulating cuprates upon cooling below the critical temperature Tc. This effect is accompanied by the appearance of the superconducting gap and a pairing peak above the gap in the Raman spectrum, and it can be understood as a hitherto-undetected feedback effect on the high-energy magnetic fluctuations due to the Cooper pairing interaction. This implies a direct involvement of the high-energy magnetic fluctuations in the pairing mechanism. All of these effects occur already above Tc in two underdoped samples, demonstrating a related feedback mechanism associated with the pseudogap.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
HgBa2CuO4+δ

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77Pressure not reportedunknown
HgBa2CuO4+δ

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

94Pressure not reportedunknown
HgBa2CuO4+δ

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

90Pressure not reportedunknown
La1.78Sr0.22CuO4

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown

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