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Ultrafast Dynamics Evidence of High Temperature Superconductivity in Single Unit Cell FeSe on SrTiO3

Y. C. Tian, W. H. Zhang, F. S. Li, Y. L. Wu, Q. Wu, F. Sun, G. Y. Zhou, Lili Wang, Xucun Ma, Qi-Kun Xue, Jimin Zhao

DOI 10.1103/PhysRevLett.116.107001 · Physical Review Letters

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Abstract

We report the time-resolved excited state ultrafast dynamics of single unit cell (1 UC) thick FeSe films on SrTiO3 (STO), with FeTe capping layers. By measuring the photoexcited quasiparticles’ density and lifetime, we unambiguously identify a superconducting (SC) phase transition, with a transition temperature Tc of 68 (−5/+2) K and a SC gap of Δ(0)=20.2±1.5 meV. The obtained electron-phonon coupling strength λ is as large as 0.48, demonstrating the likely crucial role of electron-phonon coupling in the high temperature superconductivity of the 1 UC FeSe on STO systems. We further find a 0.05 THz coherent acoustic phonon branch in the capping layer, which provides an additional decay channel to the gluing bosons.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
FeSe

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68Pressure not reportedonset
FeSe

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55Pressure not reportedunknown
FeSe

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65Pressure not reportedunknown
FeSe

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60Pressure not reportedunknown
FeSe

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58Pressure not reportedunknown
FeSe

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40Pressure not reportedunknown
FeSe

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

109Pressure not reportedunknown
FeSe

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20Pressure not reportedunknown
FeSe

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45Pressure not reportedonset

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