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Intrinsic Charge Dynamics in High-Tc AFeAs(O,F) Superconductors

A. Charnukha, D. Pröpper, N. D. Zhigadlo, M. Naito, M. Schmidt, Zhe Wang, J. Deisenhofer, A. Loidl, B. Keimer, A. V. Boris, D. N. Basov

DOI 10.1103/PhysRevLett.120.087001 · Physical Review Letters

T1

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Abstract

We report the first determination of the in-plane complex optical conductivity of 1111 high-Tc superconducting iron oxypnictide single crystals PrFeAs(O,F) and thin films SmFeAs(O,F) by means of conventional and microfocused infrared spectroscopy, ellipsometry, and time-domain THz transmission spectroscopy. A strong itinerant contribution is found to exhibit a dramatic difference in coherence between the crystal and the film. Using extensive temperature-dependent measurements of THz transmission, we identify a previously undetected 2.5-meV collective mode in the optical conductivity of SmFeAs(O,F), which is strongly suppressed at Tc and experiences an anomalous T-linear softening and narrowing below T*≈110 K≫Tc. The suppression of the infrared absorption in the superconducting state reveals a large optical superconducting gap with a similar gap ratio 2Δ/kBTc≈7 in both materials, indicating strong pairing.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
PrFeAsO0.6F0.35

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24Pressure not reportedonset
SmFeAs(O,F)

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55Pressure not reportedonset
FeSe

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65Pressure not reportedunknown

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