Multiple Charge Density Waves and Superconductivity Nucleation at Antiphase Domain Walls in the Nematic Pnictide Ba1−xSrxNi2As2
Sangjun Lee, John Collini, Stella X.-L. Sun, Matteo Mitrano, Xuefei Guo, Chris Eckberg, Johnpierre Paglione, Eduardo Fradkin, Peter Abbamonte
DOI 10.1103/PhysRevLett.127.027602 · Physical Review Letters
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Abstract
How superconductivity interacts with charge or nematic order is one of the great unresolved issues at the center of research in quantum materials. Ba1−xSrxNi2As2 (BSNA) is a charge ordered pnictide superconductor recently shown to exhibit a sixfold enhancement of superconductivity due to nematic fluctuations near a quantum phase transition (at xc=0.7) [1]. The superconductivity is, however, anomalous, with the resistive transition for 0.4<x<xc occurring at a higher temperature than the specific heat anomaly. Using x-ray scattering, we discovered a new charge density wave (CDW) in BSNA in this composition range. The CDW is commensurate with a period of two lattice parameters, and is distinct from the two CDWs previously reported in this material [1,2]. We argue that the anomalous transport behavior arises from heterogeneous superconductivity nucleating at antiphase domain walls in this CDW. We also present new data on the incommensurate CDW, previously identified as being unidirectional [2], showing that it is a rotationally symmetric “4Q” state with C4 symmetry. Our study establishes BSNA as a rare material containing three distinct CDWs, and an exciting test bed for studying coupling between CDW, nematic, and SC orders.
Source-reported materials — not catalogue approval
| Formula | Reported Tc (K) | Pressure (GPa) | Type |
|---|---|---|---|
| Ba1-xSrxNi2As2 Archive — visibility unverified Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula. | — | Pressure not reported | unknown |
| BaNi2As2 Archive — visibility unverified Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula. | — | Pressure not reported | unknown |
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