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Spin-excitation anisotropy in the bilayer iron-based superconductor CaKFe4As4

Tao Xie, Chang Liu, Frédéric Bourdarot, Louis-Pierre Regnault, Shiliang Li, Huiqian Luo

DOI 10.1103/PhysRevResearch.2.022018 · Physical Review Research

T1

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Abstract

We use polarized inelastic neutron scattering to study the spin-excitation anisotropy in the bilayer iron-based superconductor CaKFe4As4 (Tc=35 K). In the superconducting state, both odd and even L modulations of spin resonance have been observed in our previous unpolarized neutron-scattering experiments [Xie et al., Phys. Rev. Lett. 120, 267003 (2018)]. Here we find that the high-energy even mode (∼18meV) is isotropic in spin space, but the low-energy odd modes consist of a c-axis polarized mode around 9 meV along with another partially overlapped in-plane mode around 12 meV. We argue that such spin anisotropy is induced by the spin-orbit coupling in the spin-vortex-type fluctuations of this unique compound. The spin anisotropy is strongly affected by the superconductivity, where it is weak below 6 meV in the normal state and then transferred to higher energy and further enhanced in the odd modes of spin resonance below Tc.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
CaKFe4As4

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35Pressure not reportedunknown
FeSe

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8Pressure not reportedunknown
Ca1-yLayFe1-xNixAs2

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—Pressure not reportedunknown

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