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Probing the lattice anharmonicity of superconducting YBa2Cu3O7−δ via phonon harmonics

Alberto Ramos-Alvarez, Nina Fleischmann, Luciana Vidas, Alejandro Fernandez-Rodriguez, Anna Palau, Simon Wall

DOI 10.1103/PhysRevB.100.184302 · Physical Review B

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Abstract

We examine coherent phonons in a strongly driven sample of optimally-doped high temperature superconductor YBa2Cu3O7−δ. We observe a nonlinear lattice response of the 4.5 THz copper-oxygen vibrational mode at high excitation densities, evidenced by the observation of the phonon third harmonic and indicating the mode is strongly anharmonic. In addition, we observe how high-amplitude phonon vibrations modify the position of the electronic charge transfer resonance. Both of these results have important implications for possible phonon-driven nonequilibrium superconductivity.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
YBa2Cu3O7-δ

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90Pressure not reportedunknown

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