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Muon spin rotation and relaxation in Pr1−xNdxOs4Sb12: Superconductivity and magnetism in Pr-rich alloys

P.-C. Ho, D. E. MacLaughlin, M. B. Maple, Lei Shu, A. D. Hillier, O. O. Bernal, T. Yanagisawa, P. K. Biswas, Jian Zhang, Cheng Tan, S. D. Hishida, T. McCullough-Hunter

DOI 10.1103/PhysRevB.106.144508 · Physical Review B

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Abstract

The Pr-rich end 0≤x≤0.25 of the alloy series Pr1−xNdxOs4Sb12 has been studied using muon spin rotation and relaxation. The end compound PrOs4Sb12 is an unconventional heavy-fermion superconductor, which exhibits a spontaneous magnetic field associated with broken time-reversal symmetry (TRS) in the superconducting phase. No such field is observed in the Nd-doped alloys for x≥0.05, indicating that TRS has been restored. The superfluid density from the vortex-lattice field distribution is insensitive to Nd concentration for x≲0.2, indicating that TRS restoration does not have a strong effect on the superconducting state. No Nd3+ static magnetism, ordered or disordered, is found down to the lowest temperatures of measurement.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
PrOs4Sb12

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1.85Pressure not reportedunknown
Pr1-xNdxOs4Sb12

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown
Pr0.95Nd0.05Os4Sb12

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown

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