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Sharp resonant multiplet in femtosecond optical pair-breaking spectroscopy of optimally doped, underdoped, and Zn-doped YBa2Cu3O7−δ: Transient insulating regions in the superconducting state

Eric Li, R. P. Sharma, S. B. Ogale, Y. G. Zhao, T. Venkatesan, J. J. Li, W. L. Cao, C. H. Lee

DOI 10.1103/PhysRevB.65.184519 · Physical Review B

T1

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Abstract

Femtosecond optical pair breaking spectroscopy is performed on optimally doped, underdoped, and Zn-doped YBa2Cu3O7−δ (YBCO) thin films near 1.5 eV. A sharp resonant triplet fine structure is seen. The systematics of the data for the three cases brings out the key role of Cu-O plane system in the attendant processes. The peak separations are attributable to the reported phonon and magnetic excitations in the system. These results strongly suggest the presence of insulating antiferromagnetic domains in the superconducting state of these YBCO systems on a subpicosecond time scale.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
YBa2Cu3O7-δ

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90Pressure unresolvedonset
YBa2Cu3O7-δ

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

60Pressure unresolvedonset
YBa2Cu2.8Zn0.2O7

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38Pressure unresolvedonset

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