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Hole redistribution across interfaces in superconducting cuprate superlattices

C. Aruta, G. Ghiringhelli, C. Dallera, F. Fracassi, P. G. Medaglia, A. Tebano, N. B. Brookes, L. Braicovich, G. Balestrino

DOI 10.1103/PhysRevB.78.205120 · Physical Review B

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Abstract

With the aim of disentangling the role of the constituent blocks in the high-Tc cuprate superconductors we have measured x-ray absorption spectra at the Cu L3 edge on (Cu1−δCδ)Ba2CuOx (BCO), CaCuO2 (CCO), and BCO/CCO superconducting superlattices obtained by stacking in a sequence the two blocks. By observing the polarization dependence we could discriminate between the in-plane and out-of-plane hole densities. The results strongly indicate that charge is redistributed across the interfaces from the BCO charge reservoir block to the CCO infinite layer block. In the superconducting samples a relatively high density of out-of-plane holes is still present, whereas when the CCO layer thickness is excessive the holes appear to have preferential in-plane orientation and superconductivity is suppressed.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
CaCuO2

Archive — visibility unverified

Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown
(Cu1-δCδ)Ba2CuOx

Archive — visibility unverified

Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown

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