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Soft striped magnetic fluctuations competing with superconductivity in Fe1+xTe

C. Stock, E. E. Rodriguez, O. Sobolev, J. A. Rodriguez-Rivera, R. A. Ewings, J. W. Taylor, A. D. Christianson, M. A. Green

DOI 10.1103/PhysRevB.90.121113 · Physical Review B

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Abstract

Neutron spectroscopy is used to investigate the magnetic fluctuations in Fe1+xTe—a parent compound of chalcogenide superconductors. Incommensurate “stripelike” excitations soften with increased interstitial iron concentration. The energy crossover from incommensurate to stripy fluctuations defines an apparent hourglass dispersion. Application of sum rules of neutron scattering find that the integrated intensity is inconsistent with an S=1Fe2+ ground state and significantly less than S=2 predicted from weak crystal field arguments pointing towards the Fe2+ being in a superposition of orbital states. The results suggest that a highly anisotropic order competes with superconductivity in chalcogenide systems.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
Fe1+xTe1-yChy

Archive — visibility unverified

Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown
Fe1+xTe0.7Se0.3

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown
Fe1+xSeyTe1-y

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

—Pressure not reportedunknown

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