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Ultrafast dynamics in the presence of antiferromagnetic correlations in electron-doped cuprate La2−xCexCuO4±δ

I. M. Vishik, F. Mahmood, Z. Alpichshev, N. Gedik, J. Higgins, R. L. Greene

DOI 10.1103/PhysRevB.95.115125 · Physical Review B

T1

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Abstract

We used femtosecond optical pump-probe spectroscopy to study the photoinduced change in reflectivity of thin films of the electron-doped cuprate La2−xCexCuO4 (LCCO) with dopings of x=0.08 (underdoped) and x=0.11 (optimally doped). Above Tc, we observe fluence-dependent relaxation rates that begin at a temperature similar to the one where transport measurements first show signatures of antiferromagnetic correlations. Upon suppressing superconductivity with a magnetic field, it is found that the fluence and temperature dependence of relaxation rates are consistent with bimolecular recombination of electrons and holes across a gap (2ΔAF) originating from antiferromagnetic correlations which comprise the pseudogap in electron-doped cuprates. This can be used to learn about coupling between electrons and high-energy (ω>2ΔAF) excitations in these compounds and set limits on the time scales on which antiferromagnetic correlations are static.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
La2-xCexCuO4

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22Pressure not reportedunknown
La2-xCexCuO4

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

25Pressure not reportedunknown

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