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Superconductivity in a Hole-Doped Mott-Insulating Triangular Adatom Layer on a Silicon Surface

Xuefeng Wu, Fangfei Ming, Tyler S. Smith, Guowei Liu, Fei Ye, Kedong Wang, Steven Johnston, Hanno H. Weitering

DOI 10.1103/PhysRevLett.125.117001 · Physical Review Letters

T1

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Abstract

Adsorption of one-third monolayer of Sn on an atomically clean Si(111) substrate produces a two-dimensional triangular adatom lattice with one unpaired electron per site. This dilute adatom reconstruction is an antiferromagnetic Mott insulator; however, the system can be modulation doped and metallized using heavily doped p-type Si(111) substrates. Here, we show that the hole-doped dilute adatom layer on a degenerately doped p-type Si(111) wafer is superconducting with a critical temperature of 4.7±0.3 K. While a phonon-mediated coupling scenario would be consistent with the observed Tc, Mott correlations in the Sn-derived dangling-bond surface state could suppress the s-wave pairing channel. The latter suggests that the superconductivity in this triangular adatom lattice may be unconventional.

Source-reported materials — not catalogue approval

FormulaReported Tc (K)Pressure (GPa)Type
Sn

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Source-occurrence policy only; no material identity or catalogue acceptance is inferred from the formula.

4.7Pressure not reportedunknown
NaxCoO2·yH2O

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4.3Pressure not reportedunknown
Sn

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3.7Pressure not reportedunknown

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